Dr. Simon Amadeus Hinke: Research Interests and Significant Contributions
Significant contributions primarily focus on the modulation
of beta cell responsiveness to the incretin hormone, glucose-dependent insulinotropic
polypeptide (GIP), and potential therapeutic use of GIP in diabetes mellitus.
Two major aspects of GIP physiology were clarified by my research: (i) the blunted
responsiveness of the insulin-secreting beta cell to GIP in type II diabetes
may result from defective regulation of the GIP receptor in terms of desensitization,
internalization and down-regulation, and (ii) does the reduced GIP response
in type II diabetes preclude its use as a therapeutic agent? In regards to the
first point, we published two studies examining receptor desensitization and
internalization (Hinke,
SA, et al. Role of glucose in chronic desensitization of isolated rat
islets and mouse insulinoma (betaTC-3) cells to glucose-dependent insulinotropic
polypeptide. J. Endocrinol. 165:281-291, 2000 and Wheeler,
MB, Gelling, RW, Hinke, SA, et al. Characterization of the
carboxyl-terminal domain of the rat glucose-dependent insulinotropic polypeptide
(GIP) receptor. A role for serines 426 and 427 in regulating the rate of internalization.
J. Biol. Chem. 274:24593-24624, 1999.); a parallel study in our laboratory
indicated that defective expression of the GIP receptor in a rodent model of
type II diabetes was likely responsible for the blunted response to the hormone
in this disease state. This down-regulation of the GIP receptor was shown by
to be controlled by GIP itself (homologous desensitization), glucose concentration
and fatty acids [Condensed
/ Full].
Several studies were published regarding the therapeutic application
of GIP analogues in the treatment of diabetes. We designed a series of modifications
to the GIP peptide in order to (a) render the hormone resistant to inactivation
by the protease DPIV, which is the primary enzyme responsible for its degradation,
and (b) to identify the insulinotropic domains of the molecule to facilitate
synthesis of small molecular weight GIP receptor agonists. We described the
design, synthesis, DPIV resistance and biological activity of many synthetic
peptides (see CV for full
publication list). From these studies, several candidate analogues were
selected based upon their favourable attributes, and tested in vivo in normal
and diabetic rodents. Our paper published in Diabetes was not only the first
paper to show that synthetic GIP “super-agonists” have therapeutic
potential in the treatment of type II diabetes, providing proof of concept,
(and this was demonstrated in the same rodent model which exhibited a reduced
response to physiological levels of GIP because of receptor down-regulation),
but also was the result of systematic rational drug design (Hinke,
SA, et al. Dipeptidyl peptidase IV-resistant [D-Ala2]glucose-dependent
insulinotropic polypeptide (GIP) improves glucose tolerance in normal and obese
diabetic rats. Diabetes 51:652-661, 2002.). Along the same lines, another
study examined GIP, GLP-1, and enzyme resistant analogues, in parallel in vitro
and in vivo, as GLP-1 has already been proven to be a therapeutic option to
control glycemia in diabetes; this study further reinforces the need to examine
GIP in humans more closely (Hinke,
SA, et al. [Ser2]- and [(P)Ser2]-Incretin Analogs: Comparison of dipeptidyl
peptidase IV resistance and biological activities in vitro and in vivo. J. Biol.
Chem. 279: 3998-4006, 2004). The second aim, to create small molecular weight
agonist was also successful, and we discovered a novel 14 amino acid bioactive
domain of GIP, which could be used as a starting point for development of more
potent small molecular weight agonists (Hinke,
SA, et al. Identification of a bioactive domain in the amino-terminus
of glucose-dependent insulinotropic polypeptide (GIP). Biochim. Biophys. Acta
1547:143-155, 2001).
In a somewhat related field, we were the first to show that DPIV also cleaves and inactivates glucagon (Hinke, SA, et al. Dipeptidyl Peptidase IV Degradation of Glucagon : Characterization of Glucagon Degradation Products and DPIV Resistant Analogs. J. Biol. Chem. 275:3827-3834, 2000). DPIV inhibitors are currently in clinical trials as a new drug class for treating type II diabetes, acting to increase bioactive GIP and GLP-1. Our finding that DPIV also degrades glucagon indicates that drug action during the fasted state may result in undesireable side effects.
Current research is directed at elucidating nutrient regulation of beta cell function, with particular focus on nutrient deprivation versus loss of nutrient sensing.